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Creators/Authors contains: "Krohn, Jan"

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  1. ; ; ; ; ; ; (, Physical Chemistry Chemical Physics)
    Abundance spectra of (CO 2 ) N clusters up to N ≈ 500 acquired under a wide range of adiabatic expansion conditions are analyzed within the evaporative ensemble framework. The analysis reveals that the cluster stability functions display a strikingly universal pattern for all expansion conditions. These patterns reflect the inherent properties of individual clusters. From this analysis the size-dependent cluster binding energies are determined, shell and subshell closing sizes are identified, and cuboctahedral packing ordering for sizes above N ≈ 130 is confirmed. It is demonstrated that a few percent variation in the dissociation energies translates into significant abundance variations, especially for the larger clusters. 
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  2. ; ; ; ; ; ; ; ; ; ; et al (, The Journal of Physical Chemistry Letters)